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Low-dimensional antiferromagnetic fluctuations in the heavy-fermion paramagnetic ladder compound <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:msub><mml:mi>UTe</mml:mi><mml:mn>2</mml:mn></mml:msub></mml:math>

W. Knafo, G. Knebel, P. Steffens, Koji Kaneko, A. Rosuel, Jean‐Pascal Brison, J. Flouquet, D. Aoki, G. Lapertot, S. Raymond

2021Physical review. B./Physical review. B79 citationsDOIOpen Access PDF

Abstract

Inelastic-neutron-scattering measurements were performed on a single crystal of the heavy-fermion paramagnet $\mathrm{U}{\mathrm{Te}}_{2}$ above its superconducting temperature. We confirm the presence of antiferromagnetic fluctuations with the incommensurate wave-vector ${\mathbf{k}}_{1}=(0,0.57,0)$. A quasielastic signal is found, whose momentum-transfer dependence is compatible with fluctuations of magnetic moments $\ensuremath{\mu}\ensuremath{\parallel}\mathbf{a}$ with a sine-wave modulation of wave-vector ${\mathbf{k}}_{1}$ and in-phase moments on the nearest U atoms. Low dimensionality of the magnetic fluctuations, consequence of the ladder structure, is indicated by weak correlations along the direction $\mathbf{c}$. These fluctuations saturate below the temperature ${T}_{1}^{*}\ensuremath{\simeq}15\phantom{\rule{0.28em}{0ex}}\mathrm{K}$, in possible relation with anomalies observed in thermodynamic, electrical-transport, and nuclear-magnetic-resonance measurements. The absence or weakness of ferromagnetic fluctuations in our data collected at temperatures down to 2.1 K and energy transfers from 0.6 to 7.5 meV is emphasized. These results constitute constraints for models of magnetically mediated superconductivity in $\mathrm{U}{\mathrm{Te}}_{2}$.

Topics & Concepts

AntiferromagnetismParamagnetismHeavy fermionCondensed matter physicsPhysicsSuperconductivityRare-earth and actinide compoundsIron-based superconductors researchInorganic Chemistry and Materials