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<i>Gracilaria edulis</i> seaweed derived nitrogen, oxygen, and sulfur self‐doped biocarbon materials for supercapacitor applications: An investigation on the impact of acid washing and activation

Dhileepan Priyadharshini, Singaravelu Vivekanandhan

2023Energy Storage11 citationsDOIOpen Access PDF

Abstract

Abstract Seaweed biomass of Gracilaria edulis was effectively converted into biocarbon materials at 800°C for 1 hour under nitrogen gas flow atmosphere. The effect of HCl acid washing and ZnCl 2 ‐assisted chemical activation process on the physicochemical and capacitive performances was investigated and the obtained results were compared with their pristine counterpart. The formation of N, O, and S self‐doped biocarbon materials from G. edulis biomass was confirmed by carbon, hydrogen, nitrogen, and sulfur (CHNS), scanning electron microscopy‐energy dispersive X‐ray (SEM‐EDX) and X‐ray photoelectron spectroscopic (XPS) analyses. Further, the specific surface area of acid‐washed and activated biocarbon materials were respectively found to be 1100 and 774 m 2 g −1 , which are much greater than their pristine counterpart (111 m 2 g −1 ). The obtained pristine (GE‐PC), acid‐washed (GE‐AWC), and activated (GE‐AC) biocarbon materials were effectively explored as the electrode material for symmetric supercapacitor and showed the specific capacitance value of 33.9 (GE‐PC), 58.3 (GE‐AWC) and 76.5 (GE‐AC) F g −1 at 1 A g −1 using 1 M KOH electrolyte.

Topics & Concepts

NitrogenSupercapacitorX-ray photoelectron spectroscopyCarbon fibersSulfurMaterials scienceNitric acidActivated carbonOxygenElectrolyteChemical engineeringNuclear chemistryChemistryCapacitanceInorganic chemistryElectrodeOrganic chemistryComposite materialAdsorptionComposite numberMetallurgyEngineeringPhysical chemistrySupercapacitor Materials and FabricationLayered Double Hydroxides Synthesis and ApplicationsAdvanced Battery Materials and Technologies
<i>Gracilaria edulis</i> seaweed derived nitrogen, oxygen, and sulfur self‐doped biocarbon materials for supercapacitor applications: An investigation on the impact of acid washing and activation | Litcius