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Self‐Sacrificing Template Synthesis of Carbon Nanosheets Assembled Hollow Spheres with Abundant Active Fe–N<sub>4</sub>O<sub>1</sub> Moieties for Electrocatalytic Oxygen Reduction (Small 21/2023)

Fei‐Xiang Ma, Zheng‐Qi Liu, Guobin Zhang, Hong‐Shuang Fan, Yue Du, Liang Zhen, Cheng‐Yan Xu

2023Small18 citationsDOIOpen Access PDF

Abstract

Electrocatalytic Oxygen Reduction In article number 2207991, Cheng-Yan Xu and co-workers develop a self-sacrificing strategy to encapsulate single-atom Fe-N4O1 species into carbon hollow spheres assembled by ultrathin nanosheets Fe1–N–C hollow microspheres (Fe1/N-HCMs). Such highly open architecture is supposed to be an ideal platform to isolate and fully expose single metal atoms. Benifiting from the highly open architecture and abundant Fe-N4O1 active sites, the Fe1/N-HCMs exhibit excellent oxygen reduction performance.

Topics & Concepts

Materials scienceCarbon fibersOxygen reductionSPHERESOxygenMetalNanotechnologyOxygen atomOxygen reduction reactionChemical engineeringSelf-assemblyIdeal (ethics)MoleculeChemistryElectrodeElectrochemistryOrganic chemistryPhysical chemistryComposite materialMetallurgyPhysicsPhilosophyEngineeringComposite numberEpistemologyAstronomyElectrocatalysts for Energy ConversionConducting polymers and applicationsFuel Cells and Related Materials