Litcius/Paper detail

Multimode Lasing in Supercell Plasmonic Nanoparticle Arrays

Rebecca Heilmann, Kristian Arjas, Tommi K. Hakala, Päivi Törmä

2023ACS Photonics16 citationsDOIOpen Access PDF

Abstract

High Resolution Image Download MS PowerPoint Slide Multicolor light sources can be used in applications such as lighting and multiplexing signals. In photonic and plasmonic systems, one way to achieve multicolor light is via multimode lasing. To achieve this, plasmonic nanoparticle arrays are typically arranged in superlattices that lead to multiple dispersions of the single arrays coupled via the Bragg superlattice Bragg modes. Here, we show an alternative way to enable multimode lasing in plasmonic nanoparticle arrays. We design a supercell in a square lattice by leaving part of the lattice sites empty. This results in multiple dispersive branches caused by the supercell period and hence creates additional band edges that can support lasing. We experimentally demonstrate multimode lasing in such a supercell array. Furthermore, we identify the lasing modes by calculating the dispersion by combining the structure factor of the array design with an empty lattice approximation. We conclude that the lasing modes are the 74th Γ- and 106th X -point of the supercell. By tuning the square lattice period with respect to the gain emission, we can control the modes that lase. Finally, we show that the lasing modes exhibit a combination of transverse electric and transverse magnetic mode characteristics in polarization-resolved measurements.

Topics & Concepts

Lasing thresholdPlasmonMaterials scienceOptoelectronicsSuperlatticeOpticsSupercellLaserPhysicsWavelengthThunderstormMeteorologyPlasmonic and Surface Plasmon ResearchGold and Silver Nanoparticles Synthesis and ApplicationsPhotonic Crystals and Applications