Ir(<scp>iii</scp>)-Catalyzed direct C–H functionalization of <i>N</i>-phenylacetamide with α-diazo quinones: a novel strategy for producing 2-hydroxy-2′-amino-1,2′-biaryl scaffolds
Xingjun Li, Jiang Wang, Xiong Xie, Wenhao Dai, Xu Han, Kaixian Chen, Hong Liu
Abstract
α-Diazo quinones were applied in an Ir(iii)-catalyzed direct C-H functionalization assisted by N-phenylacetamide for the construction of highly functionalized 2-hydroxy-2'-amino-1,1'-biaryl scaffolds in good to excellent yields. This strategy features operational simplicity, atom- and step-economy and high efficiency.
Topics & Concepts
Surface modificationChemistryCatalysisDiazoCombinatorial chemistryStereochemistryOrganic chemistryPhysical chemistryCatalytic C–H Functionalization MethodsCyclopropane Reaction MechanismsSynthesis and Catalytic Reactions