Colossal magnetoresistance in a nonsymmorphic antiferromagnetic insulator
P. F. S. Rosa, Yuanfeng Xu, M. C. Rahn, J. C. Souza, Satya Kushwaha, L. S. I. Veiga, A. Bombardi, S. M. Thomas, M. Janoschek, E. D. Bauer, M. K. Chan, Zhijun Wang, J. D. Thompson, N. Harrison, P. G. Pagliuso, B. Andrei Bernevig, F. Ronning
Abstract
Abstract Here we investigate antiferromagnetic Eu 5 In 2 Sb 6 , a nonsymmorphic Zintl phase. Our electrical transport data show that Eu 5 In 2 Sb 6 is remarkably insulating and exhibits an exceptionally large negative magnetoresistance, which is consistent with the presence of magnetic polarons. From ab initio calculations, the paramagnetic state of Eu 5 In 2 Sb 6 is a topologically nontrivial semimetal within the generalized gradient approximation (GGA), whereas an insulating state with trivial topological indices is obtained using a modified Becke−Johnson potential. Notably, GGA + U calculations suggest that the antiferromagnetic phase of Eu 5 In 2 Sb 6 may host an axion insulating state. Our results provide important feedback for theories of topological classification and highlight the potential of realizing clean magnetic narrow-gap semiconductors in Zintl materials.