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A widely distributed phosphate-insensitive phosphatase presents a route for rapid organophosphorus remineralization in the biosphere

Ian D. E. A. Lidbury, David J. Scanlan, Andrew R. J. Murphy, Joseph A. Christie‐Oleza, Maria del Mar Aguiló‐Ferretjans, Andrew Hitchcock, Tim J. Daniell

2022Proceedings of the National Academy of Sciences109 citationsDOIOpen Access PDF

Abstract

Significance At several locations across the globe, terrestrial and marine primary production, which underpin global food security, biodiversity, and climate regulation, are limited by inorganic phosphate availability. A major fraction of the total phosphorus pool exists in organic form, requiring mineralization to phosphate by enzymes known as phosphatases prior to incorporation into cellular biomolecules. Phosphatases are typically synthesized in response to phosphate depletion, assisting with phosphorus acquisition. Here, we reveal that a unique bacterial phosphatase, PafA, is widely distributed in the biosphere and has a distinct functional role in carbon acquisition, releasing phosphate as a by-product. PafA, therefore, represents an overlooked mechanism in the global phosphorus cycle and a hitherto cryptic route for the regeneration of bioavailable phosphorus in nature.

Topics & Concepts

RemineralisationPhosphateBiospherePhosphataseChemistryEnvironmental scienceBiochemistryEcologyBiologyPhosphorylationInorganic chemistryFluoridePesticide and Herbicide Environmental StudiesMolecular Sensors and Ion DetectionArsenic contamination and mitigation
A widely distributed phosphate-insensitive phosphatase presents a route for rapid organophosphorus remineralization in the biosphere | Litcius