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Parallel spin stripes and their coexistence with superconducting ground states at optimal and high doping in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:msub><mml:mi>La</mml:mi><mml:mrow><mml:mn>1.6</mml:mn><mml:mo>−</mml:mo><mml:mi>x</mml:mi></mml:mrow></mml:msub><mml:msub><mml:mi>Nd</mml:mi><mml:mrow><mml:mn>0.4</mml:mn></mml:mrow></mml:msub><mml:msub><mml:mi>Sr</mml:mi><mml:mi>x</mml:mi></mml:msub><mml:msub><mml:mi>CuO</mml:mi><mml:mn>4</mml:mn></mml:msub></mml:mrow></mml:math>

Qianli Ma, Kirrily C. Rule, Zachary W. Cronkwright, Mirela Dragomir, Gabrielle Mitchell, Evan M. Smith, Songxue Chi, Alexander I. Kolesnikov, Matthew B. Stone, Bruce D. Gaulin

2021Physical Review Research22 citationsDOIOpen Access PDF

Abstract

Three-dimensional, commensurate long-range magnetic order in La 2 CuO 4 quickly evolves to quasi-twodimensional, incommensurate correlations upon doping with mobile holes, and superconductivity follows for x as small as 0.05 in the La 2-x Sr x /Ba x CuO 4 family of superconductors. The onset of superconductivity in these systems is known to be coincident with a remarkable rotation of the incommensurate spin order from "diagonal stripes" below x = 0.05 to "parallel stripes" above. However, little is known about the spin correlations at optimal and high doping levels, around and beyond the proposed quantum critical point for the pseudogap phase, p * . Here, we present elastic and inelastic neutron scattering measurements on single crystals of La 1.6-x Nd 0.4 Sr x CuO 4 with x = 0.125, 0.19, 0.24, and 0.26 and show that two-dimensional, quasistatic, parallel spin stripes have an onset at temperatures such that the parallel spin stripe phase extends beyond p * and envelops the entirety of superconducting ground states in this system. We also show that the elastic order parameter for parallel spin stripes at optimum doping, x = 0.19, displays an inflection point at superconducting T c , while the lowenergy dynamic spectral weight of parallel stripe fluctuations grows with decreasing temperature and saturates below T c .

Topics & Concepts

Condensed matter physicsPseudogapSuperconductivitySpin (aerodynamics)PhysicsCuprateNeutron scatteringDopingInelastic neutron scatteringQuantum spin liquidPhase (matter)Inflection pointScatteringOrder (exchange)Inelastic scatteringPhase diagramHigh-temperature superconductivitySpin waveQuantum critical pointRotation (mathematics)Ground stateHubbard modelMaterials scienceCritical point (mathematics)Physics of Superconductivity and MagnetismMagnetic and transport properties of perovskites and related materialsAdvanced Condensed Matter Physics
Parallel spin stripes and their coexistence with superconducting ground states at optimal and high doping in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:msub><mml:mi>La</mml:mi><mml:mrow><mml:mn>1.6</mml:mn><mml:mo>−</mml:mo><mml:mi>x</mml:mi></mml:mrow></mml:msub><mml:msub><mml:mi>Nd</mml:mi><mml:mrow><mml:mn>0.4</mml:mn></mml:mrow></mml:msub><mml:msub><mml:mi>Sr</mml:mi><mml:mi>x</mml:mi></mml:msub><mml:msub><mml:mi>CuO</mml:mi><mml:mn>4</mml:mn></mml:msub></mml:mrow></mml:math> | Litcius