Next-Generation Smart Carbon–Polymer Nanocomposites: Advances in Sensing and Actuation Technologies
Mubasshira, Md. Mahbubur Rahman, Md. Nizam Uddin, Mukitur Rhaman, Sourav Roy, Md Shamim Sarker
Abstract
The convergence of carbon nanomaterials and functional polymers has led to the emergence of smart carbon–polymer nanocomposites (CPNCs), which possess exceptional potential for next-generation sensing and actuation systems. These hybrid materials exhibit unique combinations of electrical, thermal, and mechanical properties, along with tunable responsiveness to external stimuli such as strain, pressure, temperature, light, and chemical environments. This review provides a comprehensive overview of recent advances in the design and synthesis of CPNCs, focusing on their application in multifunctional sensors and actuator technologies. Key carbon nanomaterials including graphene, carbon nanotubes (CNTs), and MXenes were examined in the context of their integration into polymer matrices to enhance performance parameters such as sensitivity, flexibility, response time, and durability. The review also highlights novel fabrication techniques, such as 3D printing, self-assembly, and in situ polymerization, that are driving innovation in device architectures. Applications in wearable electronics, soft robotics, biomedical diagnostics, and environmental monitoring are discussed to illustrate the transformative impact of CPNCs. Finally, this review addresses current challenges and outlines future research directions toward scalable manufacturing, environmental stability, and multifunctional integration for the real-world deployment of smart sensing and actuation systems.